Regioselective 1,3-dipolar cycloaddition of nitriles with nitrile imines generated from tetrazoles

Tomoya Miura, Kohei Hagiwara, Takayuki Nakamuro, Yuuya Nagata, Naoki Oku, Masahiro Murakami

研究成果査読

3 被引用数 (Scopus)

抄録

A synthesis of 3,5-disubstituted-1,2,4-triazoles from nitriles and 5-aryltetrazoles is reported. When 5-aryltetrazoles are triflylated in the presence of nitriles, the resulting 5-aryl-2-triflyltetrazoles thermally generate N-triflyl-nitrile imines through a sequence of ring-chain tautomerization and denitrogenation. The N-triflyl-nitrile imines immediately undergo 1,3-dipolar cycloaddition with nitriles in a regioselective manner, forming the corresponding 1,2,4-triazoles.

本文言語English
ページ(範囲)131-135
ページ数5
ジャーナルChemistry Letters
50
1
DOI
出版ステータスPublished - 1月 2021
外部発表はい

ASJC Scopus subject areas

  • 化学 (全般)

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