Theory for the ultrafast dynamics of excited clusters: Interplay between elementary excitations and atomic structure

M. E. Garcia, Harald Olaf Jeschke, I. Grigorenko, K. H. Bennemann

Research output: Contribution to journalArticle

5 Citations (Scopus)

Abstract

We present a theoretical study of the short-time relaxation of clusters in response to ultrafast excitations using femtosecond laser pulses. We analyze the excitation of different types of clusters (Hgn, Agn, Sin, C60 and Xen) and classify the relaxation dynamics in three different regimes, depending on the intensity of the exciting laser pulse. For low-intensity pulses (I < 1012 W/cm2) we determine the time-dependent structural changes of clusters upon ultrashort ionization and photodetachment. We also study the laser-induced non-equilibrium fragmentation and melting of Sin and C60 clusters, which occurs for moderate laser intensities, as a function of the pulse duration and energy. As an example for the case of high intensities (I > 1015 W/cm2), the explosion of clusters under the action of very intense ultrashort laser fields is described.

Original languageEnglish
Pages (from-to)361-371
Number of pages11
JournalApplied Physics B: Lasers and Optics
Volume71
Issue number3
DOIs
Publication statusPublished - Sep 2000
Externally publishedYes

ASJC Scopus subject areas

  • Physics and Astronomy (miscellaneous)
  • Physics and Astronomy(all)

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