Pressure effects on rattling and superconductivity in the einstein solids

Yoichi Ikeda, Yasuhiro Kawasaki, Takafumi Shinohara, Shingo Araki, Tatsuo Kobayashi, Atsushi Onosaka, Yoshihiko Okamoto, Jun Ichi Yamaura, Zenji Hiroi

Research output: Contribution to journalArticle

Abstract

Pressure effects on the rattling and superconductivity in the Einstein solids; AxV2Al20 (Ax = Ga0:2, Al0:3, and Y) are investigated by means of electrical resistivity measurements under high pressure. We observed bumps in resistivity at low temperatures only for Ga0:2 and Al0:3, which can be explained by scattering of conduction electrons by local phonons with Einstein temperatures of 8.5 and 22 K, respectively. The bumps gradually fade out with increasing pressure, and the temperature variations of resistivity for Ga0:2 and Al0:3 approach those of Y. This indicates that the low-energy local phonons in the Ga and Al compounds disappear at high pressures. We also observed T2 behavior with large A coefficients in the low-temperature limit for Ga and Al compounds, but not for Y. With increasing pressure, the A coefficient is largely suppressed, while H' c2 ≡ jdHc2=dTj Tc that also reflects the density of states at Fermi energy decreases more slowly. The T2 behavior in Ga and Al compounds probably originates from el-ph scatterings enhanced by rattling of Ga and Al atoms rather than el-el scatterings. An enhancement in the superconducting transition temperatures by the rattling is also demonstrated by comparing the pressure responses of T c between the three compounds. The enhancements of Tc and el-ph interaction λ is relatively small for these Einstein solids in contrast to those of the β-pyrochlore oxides.

Original languageEnglish
Article number063707
JournalJournal of the Physical Society of Japan
Volume82
Issue number6
DOIs
Publication statusPublished - Jun 2013

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pressure effects
superconductivity
electrical resistivity
phonons
scattering
augmentation
coefficients
conduction electrons
transition temperature
temperature
oxides
energy
atoms
interactions

Keywords

  • AVAl
  • Einstein solid
  • Electron-phonon scattering
  • Rattling
  • Resistivity
  • Superconductivity

ASJC Scopus subject areas

  • Physics and Astronomy(all)

Cite this

Pressure effects on rattling and superconductivity in the einstein solids. / Ikeda, Yoichi; Kawasaki, Yasuhiro; Shinohara, Takafumi; Araki, Shingo; Kobayashi, Tatsuo; Onosaka, Atsushi; Okamoto, Yoshihiko; Yamaura, Jun Ichi; Hiroi, Zenji.

In: Journal of the Physical Society of Japan, Vol. 82, No. 6, 063707, 06.2013.

Research output: Contribution to journalArticle

Ikeda, Y, Kawasaki, Y, Shinohara, T, Araki, S, Kobayashi, T, Onosaka, A, Okamoto, Y, Yamaura, JI & Hiroi, Z 2013, 'Pressure effects on rattling and superconductivity in the einstein solids', Journal of the Physical Society of Japan, vol. 82, no. 6, 063707. https://doi.org/10.7566/JPSJ.82.063707
Ikeda, Yoichi ; Kawasaki, Yasuhiro ; Shinohara, Takafumi ; Araki, Shingo ; Kobayashi, Tatsuo ; Onosaka, Atsushi ; Okamoto, Yoshihiko ; Yamaura, Jun Ichi ; Hiroi, Zenji. / Pressure effects on rattling and superconductivity in the einstein solids. In: Journal of the Physical Society of Japan. 2013 ; Vol. 82, No. 6.
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AB - Pressure effects on the rattling and superconductivity in the Einstein solids; AxV2Al20 (Ax = Ga0:2, Al0:3, and Y) are investigated by means of electrical resistivity measurements under high pressure. We observed bumps in resistivity at low temperatures only for Ga0:2 and Al0:3, which can be explained by scattering of conduction electrons by local phonons with Einstein temperatures of 8.5 and 22 K, respectively. The bumps gradually fade out with increasing pressure, and the temperature variations of resistivity for Ga0:2 and Al0:3 approach those of Y. This indicates that the low-energy local phonons in the Ga and Al compounds disappear at high pressures. We also observed T2 behavior with large A coefficients in the low-temperature limit for Ga and Al compounds, but not for Y. With increasing pressure, the A coefficient is largely suppressed, while H' c2 ≡ jdHc2=dTj Tc that also reflects the density of states at Fermi energy decreases more slowly. The T2 behavior in Ga and Al compounds probably originates from el-ph scatterings enhanced by rattling of Ga and Al atoms rather than el-el scatterings. An enhancement in the superconducting transition temperatures by the rattling is also demonstrated by comparing the pressure responses of T c between the three compounds. The enhancements of Tc and el-ph interaction λ is relatively small for these Einstein solids in contrast to those of the β-pyrochlore oxides.

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