Observation of intrinsic half-metallic behavior of CrO2 (100) epitaxial films by bulk-sensitive spin-resolved PES

Hirokazu Fujiwara, Masanori Sunagawa, Kensei Terashima, Tomoko Kittaka, Takanori Wakita, Yuji Muraoka, Takayoshi Yokoya

Research output: Contribution to journalArticle

1 Citation (Scopus)

Abstract

We have investigated the electronic states and spin polarization of half-metallic ferromagnet CrO2 (100) epitaxial films by bulk-sensitive spin-resolved photoemission spectroscopy with a focus on non-quasiparticle (NQP) states derived from electron-magnon interactions. We found that the averaged values of the spin polarization are approximately 100% and 40% at 40K and 300K, respectively. This is consistent with the previously reported result [H. Fujiwara et al., Appl. Phys. Lett. 106, 202404 (2015).]. At 100K, peculiar spin depolarization was observed at the Fermi level (E F), which is supported by theoretical calculations predicting NQP states. This suggests the possible appearance of NQP states in CrO2. We also compare the temperature dependence of our spin polarizations with that of the magnetization.

Original languageEnglish
JournalJournal of Electron Spectroscopy and Related Phenomena
DOIs
Publication statusAccepted/In press - Aug 5 2016

Fingerprint

Spin polarization
Epitaxial films
Depolarization
Electronic states
Photoelectron spectroscopy
Fermi level
polarization
Magnetization
Electrons
depolarization
electron scattering
photoelectric emission
magnetization
temperature dependence
Temperature
electronics
spectroscopy

Keywords

  • Bulk-sensitive spin-resolved photoemission spectroscopy
  • Electron-magnon interaction
  • Half-metallic ferromagnet
  • Non-quasiparticle state
  • Spintronics

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Radiation
  • Atomic and Molecular Physics, and Optics
  • Condensed Matter Physics
  • Spectroscopy
  • Physical and Theoretical Chemistry

Cite this

Observation of intrinsic half-metallic behavior of CrO2 (100) epitaxial films by bulk-sensitive spin-resolved PES. / Fujiwara, Hirokazu; Sunagawa, Masanori; Terashima, Kensei; Kittaka, Tomoko; Wakita, Takanori; Muraoka, Yuji; Yokoya, Takayoshi.

In: Journal of Electron Spectroscopy and Related Phenomena, 05.08.2016.

Research output: Contribution to journalArticle

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AU - Terashima, Kensei

AU - Kittaka, Tomoko

AU - Wakita, Takanori

AU - Muraoka, Yuji

AU - Yokoya, Takayoshi

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