Magnetic and dielectric properties of Tb0.5Ca 0.5MnO3

Yusuke Hiramitsu, Kenji Yoshii, Yasuhiro Yoneda, Jun'ichiro Mizuki, Akio Nakamura, Yutaka Shimojo, Yoshinobu Ishii, Yukio Morii, Naoshi Ikeda

Research output: Contribution to journalArticle

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Abstract

The magnetic and dielectric properties of a perovskite manganite Tb 0.5Ca0.5MnO3 were investigated. Magnetic measurements showed three characteristic temperatures, originating from charge ordering (∼300K), antiferromagnetic ordering (∼ 120 K), and a transition to a glassy state (∼50K). The coexistence of the charge and antiferromagnetic orderings was confirmed by powder neutron diffraction. AC dielectric measurements showed large dielectric constants larger than ∼ 1000 at approximately room temperature. The temperature dependence of the dielectric constant changed just below the charge-ordering temperature. From the analysis of tan δ, the activation energy for switching the directions of polar regions was calculated to be ∼0.09eV, which is close to the activation energy of the Mn 3d electron transfer. These results strongly suggest that the dielectric properties of this material are governed by the ordering and transfer of the Mn 3d charges.

Original languageEnglish
Pages (from-to)7171-7174
Number of pages4
JournalJapanese Journal of Applied Physics, Part 1: Regular Papers and Short Notes and Review Papers
Volume46
Issue number10 B
DOIs
Publication statusPublished - Oct 22 2007

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Dielectric properties
dielectric properties
Magnetic properties
permittivity
activation energy
magnetic properties
polar regions
magnetic measurement
neutron diffraction
alternating current
electron transfer
Permittivity
Activation energy
Temperature
temperature dependence
Neutron powder diffraction
temperature
Magnetic variables measurement
room temperature
Perovskite

Keywords

  • Charge ordering
  • Dielectric property
  • Magnetic property
  • Multlferroic
  • Perovskite

ASJC Scopus subject areas

  • Physics and Astronomy (miscellaneous)

Cite this

Magnetic and dielectric properties of Tb0.5Ca 0.5MnO3. / Hiramitsu, Yusuke; Yoshii, Kenji; Yoneda, Yasuhiro; Mizuki, Jun'ichiro; Nakamura, Akio; Shimojo, Yutaka; Ishii, Yoshinobu; Morii, Yukio; Ikeda, Naoshi.

In: Japanese Journal of Applied Physics, Part 1: Regular Papers and Short Notes and Review Papers, Vol. 46, No. 10 B, 22.10.2007, p. 7171-7174.

Research output: Contribution to journalArticle

Hiramitsu, Y, Yoshii, K, Yoneda, Y, Mizuki, J, Nakamura, A, Shimojo, Y, Ishii, Y, Morii, Y & Ikeda, N 2007, 'Magnetic and dielectric properties of Tb0.5Ca 0.5MnO3', Japanese Journal of Applied Physics, Part 1: Regular Papers and Short Notes and Review Papers, vol. 46, no. 10 B, pp. 7171-7174. https://doi.org/10.1143/JJAP.46.7171
Hiramitsu, Yusuke ; Yoshii, Kenji ; Yoneda, Yasuhiro ; Mizuki, Jun'ichiro ; Nakamura, Akio ; Shimojo, Yutaka ; Ishii, Yoshinobu ; Morii, Yukio ; Ikeda, Naoshi. / Magnetic and dielectric properties of Tb0.5Ca 0.5MnO3. In: Japanese Journal of Applied Physics, Part 1: Regular Papers and Short Notes and Review Papers. 2007 ; Vol. 46, No. 10 B. pp. 7171-7174.
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AU - Shimojo, Yutaka

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AB - The magnetic and dielectric properties of a perovskite manganite Tb 0.5Ca0.5MnO3 were investigated. Magnetic measurements showed three characteristic temperatures, originating from charge ordering (∼300K), antiferromagnetic ordering (∼ 120 K), and a transition to a glassy state (∼50K). The coexistence of the charge and antiferromagnetic orderings was confirmed by powder neutron diffraction. AC dielectric measurements showed large dielectric constants larger than ∼ 1000 at approximately room temperature. The temperature dependence of the dielectric constant changed just below the charge-ordering temperature. From the analysis of tan δ, the activation energy for switching the directions of polar regions was calculated to be ∼0.09eV, which is close to the activation energy of the Mn 3d electron transfer. These results strongly suggest that the dielectric properties of this material are governed by the ordering and transfer of the Mn 3d charges.

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