High-resolution photoemission spectro-scopy for the layered antiferromagnetic (La1-zNdz)0.46Sr0.54MnO3

Tsunehiro Takeuchi, Hiroshi Nozaki, Kazuo Soda, Takeshi Kondo, Uichiro Mizutani, Takayoshi Yokoya, Takafumi Sato, Takashi Takahashi, Shik Shin, Takayuki Muro, Yuji Saitoh, Yutaka Moritomo

Research output: Contribution to journalArticle

1 Citation (Scopus)

Abstract

High-resolution HeI photoemission spectroscopy (UPS), Mn 2p-3d resonant photoemission spectroscopy (RPES) and Mn 2p X-ray absorption spectroscopy (XAS) have been performed to investigate the electronic structure and its effect on the electrical resistivity in (La1-zNdz)0.46Sr0.54MnO3 (z = 0, 0,2, 0.6 and 1.0). It was found that in the UPS and RPES spectra the Fermi edge persisted over the temperature range 15 ≤ T ≤ 340 K regardless of the magnetic structure or the composition of the samples. The density of states at the Fermi level [N(EF)] in the samples where 0 ≤ z ≤ 0.6 was increased drastically at the Curie temperature (TC) with decreasing temperature, but essentially kept unchanged across the Néel temperature (TN). A fairly large reduction at TC and a small increase at TN in the electrical resistivity with decreasing temperature are found to be well accounted for in terms of the temperature dependence of N(EF). The presence of a finite N(EF) in the insulating Nd0.46Sr0.54MnO3 was also found. Thus the origin of the insulating behavior in this sample can be regarded as the Anderson localization associated with the small density of states and the chemical disorder between Nd and Sr.

Original languageEnglish
Pages (from-to)237-241
Number of pages5
JournalJournal of Synchrotron Radiation
Volume9
Issue number4
DOIs
Publication statusPublished - Jul 1 2002
Externally publishedYes

Fingerprint

Photoemission
photoelectric emission
Photoelectron spectroscopy
high resolution
spectroscopy
Temperature
electrical resistivity
temperature
X ray absorption spectroscopy
Magnetic structure
Curie temperature
absorption spectroscopy
Fermi level
Electronic structure
disorders
electronic structure
temperature dependence
Chemical analysis
x rays

Keywords

  • Colossal magnetoresistance
  • Manganite
  • Metal-insulator transition
  • RPES
  • UPS
  • XAS

ASJC Scopus subject areas

  • Instrumentation
  • Atomic and Molecular Physics, and Optics
  • Radiation
  • Physics and Astronomy (miscellaneous)

Cite this

High-resolution photoemission spectro-scopy for the layered antiferromagnetic (La1-zNdz)0.46Sr0.54MnO3. / Takeuchi, Tsunehiro; Nozaki, Hiroshi; Soda, Kazuo; Kondo, Takeshi; Mizutani, Uichiro; Yokoya, Takayoshi; Sato, Takafumi; Takahashi, Takashi; Shin, Shik; Muro, Takayuki; Saitoh, Yuji; Moritomo, Yutaka.

In: Journal of Synchrotron Radiation, Vol. 9, No. 4, 01.07.2002, p. 237-241.

Research output: Contribution to journalArticle

Takeuchi, T, Nozaki, H, Soda, K, Kondo, T, Mizutani, U, Yokoya, T, Sato, T, Takahashi, T, Shin, S, Muro, T, Saitoh, Y & Moritomo, Y 2002, 'High-resolution photoemission spectro-scopy for the layered antiferromagnetic (La1-zNdz)0.46Sr0.54MnO3', Journal of Synchrotron Radiation, vol. 9, no. 4, pp. 237-241. https://doi.org/10.1107/S0909049502008889
Takeuchi, Tsunehiro ; Nozaki, Hiroshi ; Soda, Kazuo ; Kondo, Takeshi ; Mizutani, Uichiro ; Yokoya, Takayoshi ; Sato, Takafumi ; Takahashi, Takashi ; Shin, Shik ; Muro, Takayuki ; Saitoh, Yuji ; Moritomo, Yutaka. / High-resolution photoemission spectro-scopy for the layered antiferromagnetic (La1-zNdz)0.46Sr0.54MnO3. In: Journal of Synchrotron Radiation. 2002 ; Vol. 9, No. 4. pp. 237-241.
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