Charge-orbital-lattice coupling effects in the d d excitation profile of one-dimensional cuprates

J. J. Lee, B. Moritz, W. S. Lee, M. Yi, C. J. Jia, A. P. Sorini, K. Kudo, Y. Koike, K. J. Zhou, C. Monney, V. Strocov, L. Patthey, T. Schmitt, T. P. Devereaux, Z. X. Shen

Research output: Contribution to journalArticle

23 Citations (Scopus)

Abstract

We identify dd excitations in the quasi-one-dimensional compound Ca 2Y2Cu5O10 using resonant inelastic x-ray scattering. By tuning across the Cu L3 edge, we observe abrupt shifts in the dd-peak positions as a function of incident photon energy. This observation demonstrates orbital-specific coupling of the high-energy excited states of the system to the low-energy degrees of freedom. A Franck-Condon treatment of electron-lattice coupling, consistent with other measurements in this compound, reproduces these shifts, explains the Gaussian line shapes, and highlights charge-orbital-lattice renormalization in the high-energy d manifold.

Original languageEnglish
Article number041104
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume89
Issue number4
DOIs
Publication statusPublished - Jan 9 2014

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

Fingerprint Dive into the research topics of 'Charge-orbital-lattice coupling effects in the d d excitation profile of one-dimensional cuprates'. Together they form a unique fingerprint.

  • Cite this

    Lee, J. J., Moritz, B., Lee, W. S., Yi, M., Jia, C. J., Sorini, A. P., Kudo, K., Koike, Y., Zhou, K. J., Monney, C., Strocov, V., Patthey, L., Schmitt, T., Devereaux, T. P., & Shen, Z. X. (2014). Charge-orbital-lattice coupling effects in the d d excitation profile of one-dimensional cuprates. Physical Review B - Condensed Matter and Materials Physics, 89(4), [041104]. https://doi.org/10.1103/PhysRevB.89.041104